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Seasonal variation of aerosol water uptake and its impact on the direct radiative effect at Ny-Alesund, Svalbard
Stockholm Univ, Dept Appl Environm Sci ITM, S-11418 Stockholm, Sweden.;Stockholm Univ, Bert Bolin Ctr Climate Res, S-11418 Stockholm, Sweden..
Lund Univ, Div Nucl Phys, SE-21100 Lund, Sweden..
Stockholm Univ, Dept Appl Environm Sci ITM, S-11418 Stockholm, Sweden.;Stockholm Univ, Bert Bolin Ctr Climate Res, S-11418 Stockholm, Sweden..
Stockholm Univ, Dept Appl Environm Sci ITM, S-11418 Stockholm, Sweden.;Stockholm Univ, Bert Bolin Ctr Climate Res, S-11418 Stockholm, Sweden..
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2014 (English)In: Atmospheric Chemistry And Physics, ISSN 1680-7316, E-ISSN 1680-7324, Vol. 14, no 14, 7445-7460 p.Article in journal (Refereed) Published
Abstract [en]

In this study we investigated the impact of water uptake by aerosol particles in ambient atmosphere on their optical properties and their direct radiative effect (ADRE, W m(-2)) in the Arctic at Ny-Alesund, Svalbard, during 2008. To achieve this, we combined three models, a hygroscopic growth model, a Mie model and a radiative transfer model, with an extensive set of observational data. We found that the seasonal variation of dry aerosol scattering coefficients showed minimum values during the summer season and the beginning of fall (July-August-September), when small particles (< 100 nm in diameter) dominate the aerosol number size distribution. The maximum scattering by dry particles was observed during the Arctic haze period (March-April-May) when the average size of the particles was larger. Considering the hygroscopic growth of aerosol particles in the ambient atmosphere had a significant impact on the aerosol scattering coefficients: the aerosol scattering coefficients were enhanced by on average a factor of 4.30 +/- 2.26 (mean +/- standard deviation), with lower values during the haze period (March-April-May) as compared to summer and fall. Hygroscopic growth of aerosol particles was found to cause 1.6 to 3.7 times more negative ADRE at the surface, with the smallest effect during the haze period (March-April-May) and the highest during late summer and beginning of fall (July-August-September).

Place, publisher, year, edition, pages
2014. Vol. 14, no 14, 7445-7460 p.
Research subject
SWEDARCTIC 2006, Zeppelin; SWEDARCTIC 2007, Zeppelin 2007
Identifiers
URN: urn:nbn:se:polar:diva-2288DOI: 10.5194/acp-14-7445-2014ISI: 000339934900018OAI: oai:DiVA.org:polar-2288DiVA: diva2:858155
Available from: 2015-10-01 Created: 2015-10-01 Last updated: 2015-10-01

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