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The importance of Aitken mode aerosol particles for cloud sustenance in the summertime high Arctic: A simulation study supported by observational data
Stockholms universitet, Meteorologiska institutionen (MISU).
Stockholms universitet, Meteorologiska institutionen (MISU).
Stockholms universitet, Meteorologiska institutionen (MISU).
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2021 (engelsk)Inngår i: Atmospheric Chemistry And Physics, ISSN 1680-7316, E-ISSN 1680-7324, Vol. 21, nr 5, s. 3871-3897Artikkel i tidsskrift (Fagfellevurdert) Published
Abstract [en]

The potential importance of Aitken mode particles (diameters similar to 25-80 nm) for stratiform mixed-phase clouds in the summertime high Arctic (> 80 degrees N) has been investigated using two large-eddy simulation models. We find that, in both models, Aitken mode particles significantly affect the simulated microphysical and radiative properties of the cloud and can help sustain the cloud when accumulation mode concentrations are low (< 10-20 cm-3), even when the particles have low hygroscopicity (hygroscopicity parameter - kappa = 0.1). However, the influence of the Aitken mode decreases if the overall liquid water content of the cloud is low, either due to a higher ice fraction or due to low radiative cooling rates. An analysis of the simulated supersaturation (ss) statistics shows that the ss frequently reaches 0.5 % and sometimes even exceeds 1 %, which confirms that Aitken mode particles can be activated. The modelling results are in qualitative agreement with observations of the Hoppel minimum obtained from four different expeditions in the high Arctic. Our findings highlight the importance of better understanding Aitken mode particle formation, chemical properties and emissions, particularly in clean environments such as the high Arctic.

sted, utgiver, år, opplag, sider
2021. Vol. 21, nr 5, s. 3871-3897
HSV kategori
Forskningsprogram
SWEDARCTIC 2008, ASCOS
Identifikatorer
URN: urn:nbn:se:polar:diva-8677DOI: 10.5194/acp-21-3871-2021ISI: 000630173500004OAI: oai:DiVA.org:polar-8677DiVA, id: diva2:1548589
Tilgjengelig fra: 2021-04-11 Laget: 2021-05-03bibliografisk kontrollert

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Igel, Adele L.Riipinen, IlonaEkman, Annica M. L.
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